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There are way more than 5 giant creatures in fallout 4. But this guide will show you where 5 of them are so you can get the trophy or achievement be sure to be well equipped to fight these guys or else they will kill you!

Its best to do these alone without a companion. If you go with a companion he might kill it instead of you and it wont count and these rare enemies dont respawn. Only mirelurks and behemoths are considered giant creatures.